I have recentered my axles with adjustable Trac bars. That and adjustable control arms have made a huge difference in handling on my jeep.
Re-centering your axle will have had NO effect in the way your Jeep handles. Your new adjustable front lower control arms can only be set at a minimum length of 23-1/16" and with the amount of lift you have, I would venture to guess that your caster is currently upwards of +5° or more (something I used to recommend). While that would have made a huge difference in the way your Jeep handles, it will effectively increase your chances of getting driveline vibrations and will lead to premature drive shaft joint failure. Just something you might want to be aware of.